Drop impact on heated surfaces

Effect of polymer additives

The impact of liquid drops on hot surfaces is a complex phenomenon which is important in various Engineering applications (spray cooling or quenching, firefighting, etc.). The impact morphology depends mainly on the surface temperature (when it exceeds the saturation temperature of the liquid), and the Weber number (which compares inertia and surface forces), as shown in the following qualitative map:

 

 

Very small amounts of flexible polymers are known to change significantly the behaviour of liquid droplets when they impact on a solid surface. This was observed for the first time at Rhodia Recherche (Lyon, France) by Vance Bergeron, who discovered that PEO suppressed drop rebound on hydrophobic surfaces. The chemical structure of these additives consists of linear of weakly branched chains of monomers, and their molecular weight is rather high (106-107 a.m.u.). A typical example is polyethylene oxide (PEO).

 

We have found that polymers also change the impact morphology of drops on heated surfaces.

 

One of the most spectacular phenomena that happen when a liquid drop hits a hot surface is the scattering of smaller secondary droplets from the free surface. See an example in the movie below on the left (T = 250°C; We = 40).

When we add to the liquid a very small amount of polyethylene oxide (200 ppm), and we repeat the experiment in the same conditions, secondary atomization completely disappears, and the drop just rebounds on the surface (see the movie below on the right).

 

         

 

For high Weber numbers, drops break down into smaller droplets upon impact (splashing); this phenomenon is enhanced by high temperatures of the surface. See an example in the movie below on the left (T = 120°C; We = 220). Polyethylene oxide (200 ppm) prevents the drop from breaking-down (see the movie below on the right).

 

         

 

V. Bertola, K. Sefiane, Controlling secondary atomization during drop impact on hot surfaces by polymer additives, Physics of Fluids, vol. 17(10), article 108104, 2005.

 

V. Bertola, Drop impact on a hot surface: effect of a polymer additive, Experiments in Fluids, vol. 37(5), pp. 653-664, 2004.