Edge instability and its interplay with bulk shear flows

 

Suzanne Fielding

Durham University, UK

 

Abstract

 

This seminar will review recent progress in understanding theoretically the edge fracture instability in sheared complex fluids, and the interplay of edge fracture with bulk shear flows.

In the most common rheological experiment, a sample of complex fluid is sandwiched between plates and sheared. Commonly encountered beyond a critical (material and device dependent) shear rate is the phenomenon of edge fracture: the free surface where the fluid sample meets the outside air destabilises, rendering accurate rheological measurement impossible. Edge fracture is often discussed as one of the most important limiting factors in rotational rheometry. From a fluid mechanical viewpoint, it is an important example of a hydrodynamic instability in a free surface viscoelastic flow.

Following a brief introduction to the basic phenomenon of edge fracture, I will present the results of recent linear stability analyses and direct nonlinear simulations of the phenomenon. An exact analytical expression will be presented for the onset of edge fracture, expressed in terms of the shear-rate derivative of the second normal stress difference, the shear-rate derivative of the shear stress, the jump in shear stress across the interface between the fluid and the outside air, the surface tension of that interface, and the rheometer gap size. Our findings also afford a full mechanistic understanding of the instability, which we have carefully validated against our simulations. They also suggest a possible route to mitigating edge fracture, potentially allowing experimentalists to achieve and accurately measure stronger flows than hitherto.

The final part of the talk will discuss the interplay of edge disturbance/instability with the bulk shear flow, with a particular focus on shear banding in the fluid bulk. (In the first part of the talk above, the bulk flow was assumed homogeneous and unbanded.) First, I will discuss how edge disturbances can induce a quasi-bulk apparent shear banding that persists far into the bulk. (To paraphrase this scenario “edge fracture causes bulk shear banding”.) Second, I will discuss opposite case, in which bulk shear banding induces edge fracture. Numerical results will then demonstrate a more general interplay between surface and bulk physics, in between these two extreme causalities.


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